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In May 2015 her first book Homeopathy Reconsidered — What Really Helps Patients was published by Springer Verlag in German (German title Homöopathie neu gedacht – Was Patienten wirklich hilft). She abandoned her homeopathic activity the same year. Grams is currently active as a science communicator.

The impact of Grams' position in print media, radio, and television was an essential factor in the intensified German public discourse surrounding homeopathy since 2015. She delivered a talk at SkepKon 2017 titled Enlightenment about pseudomedicine: What have skeptics achieved?

Grams took up the publication of her 2015 book with the intention of stimulating self-reflection among those in the homeopathic orbit. She has expressed regret that this introspection had not yet happened until today. Homeopaths who reviewed her first book didn't go to a factual discourse but have questioned the motivation behind her conversion (i.e., her change of mind based on rational arguments), mostly in a defamatory way. Grams reported that she had received a lot of rejection since becoming a public critic of homeopathy, often in the form of personal attacks, defamations, even death threats. She had even had to take advantage of police protection at events.

Instead, her research in preparation for this rebuttal caused her to reconsider the scientific evidence on the subject of homeopathy. This in turn led Grams to revise her own views on the topic. Rather than the planned defense of homeopathy, her first book Homeopathy Reconsidered — What Really Helps Patients, published in May 2015, turned out to be a critical examination of the discipline. The book is especially critical of claims that homeopathy constitutes a specific drug therapy. Grams says she tried to be empathetic in her writing style, intending for the reader to "feel [her] agony, discovering these facts about homeopathy." As a practicing homeopath, Grams had experienced individual successes in treating patients, but her search for scientific arguments to justify these successes led her to realize that little evidence existed. She described the beginning of her doubts about homeopathy as coming "…when [she] learned that, in evaluating the efficacy of a therapy, the decisive thing is not one's experience but rather the results of clinical studies." She has said that letting go of her perception of homeopathy as "some sort of 'parallel knowledge' … just as admissible and legitimate as scientific knowledge" required a realization that she had deeply deceived herself.

Although Grams fundamentally opposes homeopathy as a discipline, she wishes to see mainstream health systems embrace the idea of better medicine — an effort to enable intensive attention to the patient in daily medical practice. In interviews with German daily newspapers Süddeutsche Zeitung and Die Welt, Grams stated that "[h]omeopathy works because we homeopaths and our patients have the idea that it works", and characterized homeopathy itself as a patient which "lacks data and facts, it hallucinates, it does not want to admit its illness. But insight into illness can be a first step to recovery." She perceives a distorted picture among homeopaths of scientific work, in which science is thought to be not a method but a worldview; this misunderstanding leads to a lack of clarity about the ardour and rigor science requires in order to produce a result. She nonetheless considers the practical element of homeopathy — attentiveness to the patient — valuable, opining that physicians "must carry this over into everyday medical and clinical life — but without the magic part involving succussion and potentization." In an interview with Der Spiegel, Grams said that given the lack of evidence for homeopathic medicines' efficacy exceeding the placebo effect, "[i]f a group of doctors staunchly asserts that homeopathy works, one must — for the sake of patients — object."

Along with author and homeopathy critic Norbert Aust, Grams co-founded the Information Network on Homeopathy (Informationsnetzwerk Homöopathie — INH) in 2016.

She lent her expertise as a member of the "Münsteraner Kreis", a free association of scientists on the subject of "Pseudomedicine in Public Health",.as an author in support of the Münster Memorandum on Practitioners of Alternative Medicine, which aims to mitigate the potential for patient harm from therapists who lack academic medical education (Heilpraktiker — literally healing practitioners) by proposing a German regulatory framework to balance the concerns of patient autonomy and freedom of therapy against fairness to health insurance providers and insurees. She also co-authored the second publication of the Münsteraner Kreis, the "Münster Memorandum on Homeopathy", which appeared in 2018.

In 2004, in parallel with her medical education, Grams began pursuing education in traditional Chinese medicine and homeopathy. She completed her homeopathic education with an additional professional designation in that area, and was active exclusively in private homeopathic practice from 2009 through 2015.

Grams grew up in Bavaria, where she graduated high school in 1997. She studied medicine at Ludwig Maximilian University of Munich, Technical University of Munich, and Heidelberg University, where in 2005 she gained licensure as a physician in Germany. In 2007 she received her doctorate as a medical faculty member at the University of Zurich. Until 2009 she was an intern at a private religiously-affiliated hospital in Heidelberg, where she specialized in geriatric and palliative medicine.

Natalie Grams (born 12 April 1978) is a German physician and author. Formerly a practicing homeopath, she became known throughout Germany as a whistleblower for her 2015 debut book Homeopathy Reconsidered — What Really Helps Patients in which she criticized homeopathy. In 2016 she joined the Science Council of the Society for the Scientific Investigation of Parasciences (GWUP - the German Sceptics Association). and in January 2017 she became Communications Manager for the GWUP. She also serves on the advisory board of the humanist Giordano Bruno Foundation since May 2017, and as vice president of the Humanist Press Foundation in Germany since October 2017. In October 2017 her second book, Gesundheit — A Book Not Without Side Effects, was published.